Substantial gadolinium enrichments in lake and river near metrocities in Korea

Title
Substantial gadolinium enrichments in lake and river near metrocities in Korea
Author(s)
Kim, Intae; Kim, Suk Hyun
KIOST Author(s)
Kim, In Tae(김인태)Kim, Suk Hyun(김석현)
Publication Year
2020-05-05
Abstract
We measured dissolved rare earth elements (REEs) in the water samples from Shihwa Lake (SL), which was assumed to be highly polluted, as well as in the downstream portion of the Han River (HR), which runs through, Seoul, Korea. Among the investigated REEs, only Gadolinium (Gd) was found to be significantly enhanced after REE concentrations were shale-normalized (SN). The calculated Gd anomaly (Gd/Gd* = 3×GdSN/(SmSN + 2×TbSN)) was about 1.5±0.1 (n=16) in SL and 1.6±0.3 in HR (n=26) water relative to other types of natural water such as groundwater, seawater, and river water in uncontaminated areas (Gd/Gd*~1.2, n>400). These significant Gd anomalies seem to be due to the inputs of anthropogenic Gd (Gdanth), especially by the use of Gd-based contrast agents for magnetic resonance imaging (MRI) tests from a number of hospitals and medical institutes surrounding our study areas. The Gdanth inventory was estimated to be 190±80 g and 680±360 kg Gd in SL and the HR (watersheds in our study area), respectively. The Gdanth flux to the Yellow Sea from the HR is estimated to be 530±330 g Gd day-1. Overall, these results suggest that quantitative evaluation of man-made REEs for associated human risk assessments are needed, because considerable amounts of REEs are now used by modern high-tech industries.
URI
https://sciwatch.kiost.ac.kr/handle/2020.kiost/37702
Bibliographic Citation
The EGU General Assembly 2020, 2020
Publisher
European Geoscience Union
Type
Conference
Language
English
Publisher
European Geoscience Union
Related Researcher
Research Interests

marine pollution management,marine biogeochemistry,marine environmental radioactivity,해양오염관리,해양물질순환,해양환경방사능

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